基于优势手性片段策略的配体设计及在烯烃不对称氢芳基化反应和聚合反应中的应用

91856111
2018
B0106.不对称合成
施世良
重大研究计划
研究员
中国科学院上海有机化学研究所
75万元
高分子手性;不对称碳碳键形成;手性配体;不对称金属催化;不对称碳氢键活化
2019-01-01到2021-12-31
  • 中英文摘要
  • 结题摘要
  • 结题报告
  • 项目成果
  • 项目参与人
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序号 标题 类型 作者
1 Aluminum-Catalyzed Selective Hydroboration of Alkenes and Alkynylsilanes 期刊论文 Li Feng Bai Xu Cai Yuan Li Han Zhang Shuo-Qing Liu Feng-Hua Hong Xin Xu Youjun;Shi Shi-Liang
2 A Bulky Chiral N-Heterocyclic Carbene Palladium Catalyst Enables Highly Enantioselective Suzuki-Miyaura Cross-Coupling Reactions for the Synthesis of Biaryl Atropisomers. 期刊论文 Di Shen;Youjun Xu;Shi-Liang Shi
3 Fast Enantio- and Chemoselective Arylation of Ketones with Organoboronic Esters Enabled by Nickel/N-Heterocyclic Carbene Catalysis 期刊论文 Yuan Cai;Lin-Xin Ruan;Abdul Rahman;Shi-Liang Shi
4 镍催化的丁二烯、醛、炔和氢氯二茂锆的多组分偶联反应合成1,4-二烯 期刊论文 李雨青;施世良
5 Regio- and Enantioselective C-H Cyclization of Pyridines with Alkenes Enabled by a Nickel/N-Heterocyclic Carbene Catalysis. 期刊论文 Wu-Bin Zhang;Xin-Tuo Yang;Jun-Bao Ma;Zhi-Ming Su;Shi-Liang Shi
6 Thieme Chemistry Journals Award 奖励 Shi-Liang Shi
7 Enantioconvergent Arylation of Racemic Secondary Alcohols to Chiral Tertiary Alcohols Enabled by Nickel/N-Heterocyclic Carbene Catalysis 期刊论文 Cai Yuan;Shi Shi-Liang
8 nBuLi-promoted anti-Markovnikov selective hydroboration of unactivated alkenes and internal alkynes 期刊论文 Wang Zi-Chao Wang Min Gao Jian Shi Shi-Liang;Xu Youjun
9 Enantioselective Ni/N-Heterocyclic Carbene-Catalyzed Redox- Economical Coupling of Aldehydes, Alkynes, and Enones for Rapid Construction of Acyclic All-Carbon Quaternary Stereocenters 期刊论文 Wu-Bin Zhang;Guang Chen;Shi-Liang Shi
10 手性1,3-二芳基咪唑盐卡宾前体、其合成方法、金属盐复合物和应用 专利 施世良;蔡援;杨新拓;李峰
11 Low-Temperature Nickel-Catalyzed C-N Cross-Coupling via Kinetic Resolution Enabled by a Bulky and Flexible Chiral N-Heterocyclic Carbene Ligand 期刊论文 Wang Zi-Chao;Xie Pei-Pei;Xu Youjun;Hong Xin;Shi Shi-Liang
12 Nickel/NHC-Catalyzed Asymmetric C-H Alkylation of Fluoroarenes with Alkenes: Synthesis of Enantioenriched Fluorotetralins. 期刊论文 Yuan Cai;Xiaodong Ye;Sheng Liu;Shi-Liang Shi
13 Regio- and Trans-Selective Ni-Catalyzed Coupling of Butadiene, Carbonyls, and Arylboronic Acids to Homoallylic Alcohols under Base-Free Conditions 期刊论文 Yu-Qing Li;Guang Chen;Shi-Liang Shi
14 Ni-Catalyzed Coupling of Butadiene, Aldimines, and Arylboronic Acids to Homoallylic Amines under Base-Free Conditions 期刊论文 Li Yu-Qing;Shi Shi-Liang
15 Ni-Catalyzed Three-Component Coupling Reaction of Butadi- ene, Aldimines and Alkenylboronic Acids 期刊论文 Zhang Yurong;Wang Han;Mao Yongjun;Shi Shi-Liang
16 钯复合物、其制备方法、轴手性联芳香化合物的制备方法 专利 施世良;申迪
17 Nickel/NHC-Catalyzed Enantioselective Cyclization of Pyridones and Pyrimidones with Tethered Alkenes 期刊论文 Di Shen;Wu-Bin Zhang;Zhiyang Li;Shi-Liang Shi;Youjun Xu
18 Base-catalysed reductive relay hydroboration of allylic alcohols with pinacolborane to form alkylboronic esters. 期刊论文 Wang Zi-Chao;Shen Di;Gao Jian;Jia Xian;Xu Youjun;Shi Shi-Liang
19 Nickel-Catalyzed Ligand-Free Hiyama Coupling of Aryl Bromides and Vinyltrimethoxysilane 期刊论文 Shichao Wei;Yongjun Mao;Shi-Liang Shi
20 Base-Promoted Rapid Hydrosilylation of Aldimine 期刊论文 Zi-Chao Wang;Youjun Xu;Shi-Liang Shi
21 Ligand- and Additive-Free CuCl 2 -Catalyzed para-C-H Alkylation of Aniline Derivatives via Carbene Insertion 期刊论文 Lei Gao;Sheng Liu;Zi-Chao Wang;Yongjun Mao;Shi-Liang Shi
22 Expedient Synthesis of Ketones via N-Heterocyclic Carbene/ Nickel-Catalyzed Redox-Economical Coupling of Alcohols and Alkynes 期刊论文 Yu-Qing Li;Feng Li;Shi-Liang Shi
23 ChemComm Emerging Investigator 奖励 Shi-Liang Shi
24 Chemo-andEnantioselectiveArylation andAlkenylationofAldehydesEnabled by Nickel/N-Heterocyclic Carbene Catalysis 期刊论文 Zi-Chao Wang;Jian Gao;Yuan Cai;Xiaodong Ye;Shi-Liang Shi
25 Bayer Investigate Award 奖励 Shi-Liang Shi
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