【21272222】新型含氮双官能团催化剂的设计及其在不对称合成中的应用国家自然基金项目

新型含氮双官能团催化剂的设计及其在不对称合成中的应用

项目批准号： 21272222

批准年份： 2012

学科分类： B0106.不对称合成

项目负责人：汪志勇

资助类别：面上项目

负责人职称：教授

依托单位：中国科学技术大学

资助金额： 80万元

关键词：催化剂;设计;不对称合成;含氮配体;双功能团

起止时间： 2013-01-01到2016-12-31

中英文摘要
结题摘要
结题报告
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序号	标题	类型	作者
1	Cerium(III)-catalyzed cascade cyclization: an efficient approach to functionalized pyrrolo[1,2-a]quinolines	期刊论文	Yan, Yizhe\|Zhang, Zhenglei\|Xu, Kun\|Wang, Zhiyong\|
2	Catalyst-free sulfonylation of activated alkenes for highly efficient synthesis of mono-substituted ethyl sulfones in water	期刊论文	Zhang, Sheng\|Guo, Xuefeng\|Zha, Zhenggen\|Wang, Zhiyong\|
3	Asymmetric Formal Aza-Diels-Alder Reaction of Trifluoromethyl Hemiaminals with Enones Catalyzed by Primary Amines	期刊论文	Hu, Yanbin\|Li, Yanan\|Zha, Zhenggen\|Wang, Zhiyong\|
4	Copper-Catalyzed Enantioselective Friedel-Crafts Alkylation of Pyrrole with Isatins	期刊论文	Zhang, Sheng\|Hu, Yanbin\|Zha, Zhenggen\|Wang, Zhiyong\|
5	Electrochemical synthesis of alpha-enaminones from aryl ketones	期刊论文	Qian, Peng\|Bi, Meixiang\|Zha, Zhenggen\|Wang, Zhiyong\|
6	Copper-Catalyzed Radical Methylation/C-HAmination/Oxidation Cascade for the Synthesis of Quinazolinones	期刊论文	鲍亚捷\|汪志勇\|
7	A Highly Tunable Stereoselective Dimerization of Methyl Ketone: Efficient Synthesis of E- and Z-1,4-Enediones	期刊论文	Fang, Yang\|Yan, Zicong\|Zha, Zhenggen\|Wang, Zhiyong\|
8	Highly Diastereo- and Enantioselective MichaelAddition of Nitroalkanes to 2-Enoyl-Pyridine N-Oxides Catalyzed byScandium(III)/Copper(II) Complexes	期刊论文	李丽君\|汪志勇\|
9	Gold nanoparticles supported on titanium dioxide: an efficient catalyst for highly selective synthesis of benzoxazoles and benzimidazoles	期刊论文	Guo, Xuefeng\|Yang, Yu\|Zha, Zhenggen\|Wang, Zhiyong\|
10	Efficient synthesis of 2-arylquinazolines viacopper-catalyzed dual oxidative benzylic C-H aminations of methylarenes	期刊论文	刘立岩\|汪志勇\|
11	Resuable Catalysis for Copper-Mediated Cross-coupling Reactions under Heterogeneous conditions	专著	Wan, Changfeng\|Wang, Ye\|Wang, Zhiyong\|
12	Metal-Organic Framework with Functional Amide Groups for Highly Selective Gas Separation	期刊论文	He, Yabing\|Krishna, Rajamani\|Chen, Banglin\|Wang, Zhiyong\|
13	Supported gold-catalyzed and ammonia-promotedselective synthesis of quinazolines in aqueous media	期刊论文	唐林\|汪志勇\|
14	A green and efficient access to aryl nitriles via an electrochemical anodic oxidation	期刊论文	Ye\|Jia-Qian\|
15	Ligand-Free Pd-Catalyzed Domino Synthesis of Carbazoles via Dehydrogenative Aromatization/C(sp(2))-C(sp(2)) Coupling Sequence	期刊论文	Tang, Lin\|Yang, Yu\|Zha, Zhenggen\|Wang, Zhiyong\|
16	Bismuth nanoparticles: an e？cient catalystforreductive coupling of nitroarenes to azo-compounds	期刊论文	K. Pothula\|汪志勇\|
17	A novel approach for the one-pot preparation of alpha-ketoamides by anodic oxidation	期刊论文	Zhang, Zhenlei\|Su, Jihu\|Zha, Zhenggen\|Wang, Zhiyong\|
18	Catalyst-free thiolation of indoles with sulfonyl hydrazides for the synthesis of 3-sulfenylindoles in water	期刊论文	Tang, Lin\|Hu, Yanbin\|Zha, Zhenggen\|Wang, Zhiyong\|
19	Easily Accessible and Highly Tunable Bisphosphine Ligands for Asymmetric Hydroformylation of Terminal and Internal Alkenes	期刊论文	Xu\|Kun\|
20	CuI-catalyzed and air promoted oxidative cyclization for one-pot synthesis of polyarylated oxazoles	期刊论文	Yan, Yizhe\|Zhang, Shuai\|Zhang, Baiqun\|Wang, Zhiyong\|
21	Oxidative coupling of methylamine with an aminyl radical: direct amidation catalyzed by I-2/TBHP with HCl	期刊论文	Gao, Lingfeng\|Tang, Haoming\|Wang, Zhiyong\|
22	Catalyst-free radical fluorination of sulfonyl hydrazides in water	期刊论文	Yang, Yu\|Wen, Lixian\|Yang, Xingkun\|Wang, Zhiyong\|
23	Copper-Catalyzed Enantioselective Hetero-Diels-Alder Reaction of Danishefsky's Diene with Glyoxals	期刊论文	Sun, Jianan\|Li, Lijun\|Zha, Zhenggen\|Wang, Zhiyong\|
24	Fluorescence Polarization for the Evaluation of SmallMolecule Inhibitors of PCAF BRD/Tat-AcK50 Association	期刊论文	Zhang, Baiqun\|Zhang, Shuai\|Wang, Qiang\|Wang, Zhiyong\|
25	实用有机化学实验高级教程	专著	汪志勇\|
26	A simple and efficient approach to realize difunctionalization of arylketones with malonate esters via electrochemical oxidation	期刊论文	Zha, Zhenggen\|Zhang, Zhenlei\|Ma, Huanyue\|Wang, Zhiyong\|
27	Electrosynthesis of oxadiazoles from benzoylhydrazines	期刊论文	Zha, Zheng-Gen\|Zhang, Zhen-Lei\|Meng, Li\|Wang, Zhiyong\|
28	HighlyEnantioselective Construction of Fluoroalkylated Quaternary Stereocenters viaOrganocatalytic Dehydrated Mannich Reaction of Unprotected Hemiaminals withKetones	期刊论文	张胜\|汪志勇\|
29	An efficient synthesis of amides from alcohols and azides catalyzed by a bifunctional catalyst Au/DNA under mild conditions	期刊论文	Tang, Lin\|Yang, Yu\|Zha, Zhenggen\|Wang, Zhiyong\|
30	Iron-Catalyzed Synthesis of 2-Vinylquinolines via sp(3) C-H Functionalization and Subsequent C-N Cleavage	期刊论文	Li, Yunfeng\|Guo, Fengfeng\|Zha, Zhenggen\|Wang, Zhiyong\|
31	Copper Catalyzed Enantioselective Alkylation ofPyrrole with β,γ-Unsaturated α-Ketoesters: Application to One-Pot Constructionof the Seven-Membered Ring by Merging a Gold Catalysis	期刊论文	胡彦斌\|汪志勇\|
32	Electrochemical Synthesis of the Aryl alpha-Ketoesters from Acetophenones Mediated by KI	期刊论文	Zhang\|Zhenlei\|
33	Copper-catalyzed S-methylation of sulfonyl hydrazides with TBHP for the synthesis of methyl sulfones in water	期刊论文	Wang Zhiyong\|
34	Cobalt-catalyzed oxidative [3+2] cycloaddition reactions: an efficient synthesis of pyrrolo- and imidazo-[2,1-a]isoquinolinest	期刊论文	Su, Ji-Hu\|(Yan, Yizhe\|Guo, Fengfeng\|Wang, Zhiyong\|
35	.Electrosynthesis of enaminones directly from methylketones and amines with nitromethane as a carbon source	期刊论文	徐坤\|汪志勇\|
36	Copper-Catalyzed Enantioselective Hetero-Diels-Alder Reaction of Danishefsky's Diene with beta,gamma-Unsaturated alpha-Ketoesters	期刊论文	Zhang, Sheng\|Guo, Fengfeng\|Zha, Zhenggen\|Wang, Zhiyong\|
37	Synthesis of Chromones through LiOtBu/Air-Mediated Oxidation and Regioselective Cyclization of o-Hydroxyphenyl Propargyl Carbinols	期刊论文	Zhang, Baiqun\|Gao, Lingfeng\|Zha, Zhenggen\|Wang, Zhiyong\|
38	Asymmetric Michael Reaction Catalyzed by Proline Lithium Salt: Efficient Synthesis of L-Proline and Isoindoloisoquinolinone Derivatives	期刊论文	Zhang, Sheng\|Hu, Yanbin\|Zha, Zhenggen\|Wang, Zhiyong\|
39	Direct Electrosynthesis of Ketones from Benzylic Methylenes by Electrooxidative C-H Activation	期刊论文	Zha, Zhenggen\|Zhang, Li\|Zhang, Zhenlei\|Wang, Zhiyong\|
40	An efficient iron-promoted synthesis of 6H-indolo [2,3-b]quinolines and neocryptolepine derivatives	期刊论文	Yan, Zicong\|Wan, Changfeng\|Wan, Jianyong\|Wang, Zhiyong\|
41	Bifunctional Amino Sulfonohydrazide Catalyzed DirectAsymmetric Mannich Reaction of Cyclic Ketimines with Ketones: Highly Diastereo-and Enantioselective Construction of Quaternary Carbon Stereocenters	期刊论文	张胜\|汪志勇\|

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