SAPO-34分子筛催化甲醇及其衍生物转化初始C-H键活化和C-C键生成及自催化反应机制
91745109
2017
B0202.催化化学
魏迎旭
重大研究计划
研究员
中国科学院大连化学物理研究所
75万元
二甲醚;甲醇转化;C-H键活化;第一个C-C键;分子筛
2018-01-01到2020-12-31
- 中英文摘要
- 结题摘要
- 结题报告
- 项目成果
- 项目参与人
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| 序号 | 标题 | 类型 | 作者 |
|---|---|---|---|
| 1 | Capture and identification of coke precursors to elucidate the deactivation route of the methanol-to-olefin process over H-SAPO-34 | 期刊论文 | Yu Bowen;Zhang Wenna;Wei Yingxu;Wu Xinqiang;Sun Tantan;Fan Benhan;Xu Shutao;Liu Zhongmin |
| 2 | Insight into the deactivation mode of methanol-to-olefins conversion over SAPO-34: Coke, diffusion, and acidic site accessibility | 期刊论文 | Shushu Gao;Shutao Xu;Yingxu Wei;Qinglong Qiao;Zhaochao Xu;Xinqiang Wu;Mozhi Zhang;Yanli He;Shuliang Xu;Zhongmin Liu |
| 3 | Simultaneous Evaluation of Reaction and Diffusion over Molecular Sieves for Shape-Selective Catalysis | 期刊论文 | Han Jingfeng;Liu Zhiqiang;Li Hua;Zhong Jiawei;Zhang Wenna;Huang Jindou;Zheng Anmin;Wei Yingxu;Liu Zhongmin |
| 4 | Tuning the product selectivity of SAPO-18 catalysts in MTO reaction via cavity modification | 期刊论文 | Jiawei Zhong;Jingfeng Han;Yingxu Wei;Shutao Xu;Tantan Sun;Shu Zeng;Xinwen Guo;Chunshan Song;Zhongmin Liu |
| 5 | Increasing the selectivity to ethylene in the MTO reaction by enhancing diffusion limitation in the shell layer of SAPO-34 catalyst. | 期刊论文 | Jiawei Zhong;Jingfeng Han;Yingxu Wei;Shutao Xu;Yanli He;Yijun Zheng;Mao Ye;Xinwen Guo;Chunshan Song;Zhongmin Liu |
| 6 | Methanol to Olefins Reaction over Cavity-type Zeolite: Cavity Controls the Critical Intermediates and Product Selectivity | 期刊论文 | Wenna Zhang;Jingrun Chen;Shutao Xu;Yueying Chu;Yingxu Wei;Yuchun Zhi;Jindou Huang;Anmin Zheng;Xinqiang Wu;Xiangju Meng;Fengshou Xiao;Feng Deng;Zhongmin Liu |
| 7 | The template-assisted zinc ion incorporation in SAPO-34 and the enhanced ethylene selectivity in MTO reaction | 期刊论文 | Jiawei Zhong;Jingfeng Han;Yingxu Wei;Shutao Xu;Tantan Sun;Xinwen Guo;Chunshan Song;Zhongmin Liu |
| 8 | Methylcyclopentenyl cation mediated reaction route in methanol-to-olefins reaction over H-RUB-50 with small cavity | 期刊论文 | Zhang Wenna;Xu Shutao;Zhi Yuchun;Wei Yingxu;Liu Zhongmin |
| 9 | Enhancing ethylene selectivity in MTO reaction by incorporating metal species in the cavity of SAPO-34 catalysts | 期刊论文 | Jiawei Zhong;Jingfeng Han;Yingxu Wei;Shutao Xu;Tantan Sun;Xinwen Guo;Chunshan Song;Zhongmin Liu |
| 10 | 一种催化剂重积碳物种结构的定性检测方法 | 专利 | 郅玉春;王男;魏迎旭;刘中民;吴仁安;万丽红;王莉 |
| 11 | Differentiating Diffusivity in Different Channels of ZSM-5 Zeolite by Pulsed Field Gradient (PFG) NMR | 期刊论文 | Zeng Shu;Xu Shutao;Gao Shushu;Gao Mingbin;Zhang Wenna;Wei Yingxu;Liu Zhongmin |
| 12 | Cavity-controlled diffusion in 8-membered ring molecular sieve catalysts for shape selective strategy | 期刊论文 | Shushu Gao;Zhiqiang Liu;Shutao Xu;Anmin Zheng;Pengfei Wu;Bing Li;Xiaoshuai Yuan;Yingxu Wei;Zhongmin Liu |
| 13 | 一种有甲醇和共进料物种制备环戊二烯类化合物的方法 | 专利 | 于博文;张雯娜;魏迎旭;徐舒涛;刘中民 |
| 14 | 一种由醇类原料制备晕苯类化合物的方法 | 专利 | 王男;郅玉春;魏迎旭;刘中民;桑石云 |
| 15 | Methylcyclopentenyl Cations Linking Initial Stage and Highly Efficient Stage in Methanol-to-Hydrocarbon Process | 期刊论文 | Zhang Wenna;Zhang Mozhi;Xu Shutao;Gao Shushu;Wei Yingxu;Liu Zhongmin |
| 16 | 甲醇制烯烃过程第一个C-C键生成的直接机理 | 奖励 | 魏迎旭;武新强;徐舒涛;刘中民 |
| 17 | Molecular elucidating of an unusual growth mechanism for polycyclic aromatic hydrocarbons in confined space | 期刊论文 | Wang Nan;Zhi Yuchun;Wei Yingxu;Zhang Wenna;Liu Zhiqiang;Huang Jindou;Sun Tantan;Xu Shutao;Lin Shanfan;He Yanli;Zheng Anmin;Liu Zhongmin |
| 18 | Evolution of C-C Bond Formation in the Methanol-to-Olefins Process: From Direct Coupling to Autocatalysis | 期刊论文 | Xinqiang Wu;Shutao Xu;Yingxu Wei;Wenna Zhang;Jindou Huang;Shuliang Xu;Yanli He;Shanfan Lin;Tantan Sun;Zhongmin Liu |
| 19 | 一种利用分子筛催化剂制备晕苯类化合物的方法 | 专利 | 王男;郅玉春;魏迎旭;刘中民;桑石云 |
| 20 | Methanol to olefins reaction route based on methyl-cyclopentadienes as critical intermediates | 期刊论文 | Wenna Zhang;Yuchun Zhi;Jindou Huang;Xinqiang Wu;Shu Zeng;Shutao Xu;Anmin Zheng;Yingxu Wei;Zhongmin Liu |
| 21 | 一种表层富集碱性分子的分子筛材料、其制备方法及应用 | 专利 | 孙毯毯;徐舒涛;魏迎旭;刘中民;韩晶峰;桑石云 |
| 22 | Water‐Induced Structural Dynamic Process in Molecular Sieve under Mild Hydrothermal Conditions: A Novel Ship‐in‐Bottle Strategy for Acidity Identification and Catalyst Modification | 期刊论文 | Tantan Sun;Shutao Xu;Dong Xiao;Zhiqiang Liu;Guangchao Li;Anmin Zheng;Wenjuan Liu;Zhaochao Xu;Yi Cao;Qiang Guo;Nan Wang;Yingxu Wei;Zhongmin Liu |
| 23 | 测定小孔分子筛酸性的方法及应用 | 专利 | 张雯娜;孙毯毯;徐舒涛;魏迎旭;刘中民;桑石云 |
| 24 | 一种金属改性SAPO-34分子筛的制备方法及其应用 | 专利 | 钟家伟;魏迎旭;刘中民;韩晶峰;桑石云 |
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